This article discusses the correlation between the microstructural and mechanical changes in the dual-matrix Al-Ni/SiC composites processed by Accumulative Roll Bonding (ARB) technique. Three different SiC concentrations, 1, 3, and 5% were considered to reinforce Al and Al-Ni dual-matrix composites. ARB process was applied up to 7 cycles to manufacture a composite with homogenous dispersion of the three phases. The results showed that the presence of Ni layer between Al and SiC particles enhanced the dispersion of SiC in the matrix, which positively affect the mechanical strength. The maximum tensile achieved was 257 MPa for composite containing 3 % SiC after 7 ARB cycles compared to 37.2 MPa for the AA1050. Increasing SiC content reduces the adhesion between Al and Ni layers, which reduces the elasticity of the composites. However, for the composites with 5% SiC, after 3 ARB cycles, the strength was reduced due to the cracking of the Ni layer caused by the stress concentration around the SiC particles. The hardness values of the ARBed AA1050, AA1050-Ni, and AA1050-Ni/5 wt% SiC are 85.5, 93.5, and 109.7, respectively, after 7 ARB cycles. In terms of strength, the samples with 3% SiC content showed the optimum stress enhancement with minimum reduction in the elongation, which achieve a compromised response for many applications.