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Factors affecting the corrosion behaviour of aluminium in acid solutions. I. Nitrogen and/or sulphur-containing organic compounds as corrosion inhibitors for Al in HCl solutions
Faculty
Science
Year:
2013
Type of Publication:
Article
Pages:
1-13
Authors:
Abd El Haleem, S. M, Abd El Wanees, S, Abd El Aal, E. E, Farouk, A
DOI:
10.1016/j.corsci.2012.03.021
Journal:
CORROSION SCIENCE PERGAMON-ELSEVIER SCIENCE LTD
Volume:
68
Research Area:
Materials Science; Metallurgy \& Metallurgical Engineering
ISSN
ISI:000315013300001
Keywords :
Aluminum, Thermometry, Hydrogen evolution, Open circuit potential, Galvanostatic polarization, Acid corrosion
Abstract:
The corrosion behaviour of Al in 2 M HCl solution in the absence and presence of phenylhydrazine, urea, thiourea, N-allylthiourea, and thiosemicarbazide is investigated using different chemical and electrochemical techniques. The inhibition efficiencies of these compounds increase with increasing their concentration and molecular weights. The inhibitive action of these compounds is discussed in terms of blocking the electrode surface by adsorption of the inhibitor molecules according to Langmuir isotherm. The thermodynamic parameters K-ads and Delta G degrees(ads) are calculated and discussed. The values of Delta G degrees(ads) reveal strong physisorption of the inhibitors on the metal surface. (C) 2012 Elsevier Ltd. All rights reserved.
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